In predominantly Muslim Syria, the Catholic Church helps all people in need through its charitable organizations but is particularly active in the area of Homs and Aleppo, the council said in a press release.
The Pope also earmarked the collection to be taken up at his Holy Thursday evening Mass April 5 for use for humanitarian aid to Syrian refugees.
Syria's government has been fighting a yearlong uprising inspired by pro-democracy movements in Tunisia, Egypt and Libya. The United Nations says thousands of people have been killed in the conflict, and thousands more have been detained and displaced.